Yes, untunes is a Scrabble word!
...and is worth 7 points in Scrabble, and 11 points in Words with Friends
untunes
Verb
1. Cause to lose one's composure
2. Cause to be out of tune
What Scrabble words can I make with the letters in untunes?
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Words that can be created with an extra letter added to untunes:
G:unguents