Yes, align is a Scrabble word!
...and is worth 6 points in Scrabble, and 9 points in Words with Friends
align
Verb
1. Place in a line or arrange so as to be parallel or straight
2. Be or come into adjustment with
3. Align oneself with a group or a way of thinking
4. Bring (components or parts) into proper or desirable coordination correlation
What Scrabble words can I make with the letters in align?
5 Letter Words
4 Letter Words
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3 Letter Words
2 Letter Words